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Solution-processed cesium hexabromopalladate(IV), Cs2PdBr6, for optoelectronic applications

Abstract:

Lead halide perovskites are materials with excellent optoelectronic and photovoltaic properties. However, some hurdles remain prior to commercialization of these materials, such as chemical stability, phase stability, sensitivity to moisture, and potential issues due to the toxicity of lead. Here, we report a new type of lead-free perovskite related compound, Cs2PdBr6. This compound is solution processable, exhibits long-lived photoluminescence, and an optical band gap of 1.6 eV. Density func...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1021/jacs.6b13258

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Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Condensed Matter Physics
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Condensed Matter Physics
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Materials
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Condensed Matter Physics
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Inorganic Chemistry
Role:
Author
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More from this funder
Funding agency for:
Filip, MR
Grant:
EP/J009857/1
More from this funder
Funding agency for:
Filip, MR
Grant:
EP/J009857/1
More from this funder
Funding agency for:
Filip, MR
Grant:
EP/J009857/1
More from this funder
Funding agency for:
Giustino, F
Grant:
EP/J009857/1
More from this funder
Funding agency for:
Giustino, F
Grant:
EP/J009857/1
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Publisher:
American Chemical Society Publisher's website
Journal:
Journal of the American Chemical Society Journal website
Volume:
139
Issue:
17
Pages:
6030-6033
Publication date:
2017-04-20
Acceptance date:
2017-04-20
DOI:
EISSN:
1520-5126
ISSN:
0002-7863
Source identifiers:
690846
Language:
English
Pubs id:
pubs:690846
UUID:
uuid:f2e6cb07-9d8f-4ac2-adf2-106b98ca3165
Local pid:
pubs:690846
Deposit date:
2017-07-04

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