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Marcus theory of thermoelectricity in molecular junctions

Abstract:

Thermoelectric energy conversion is perhaps the most promising of the potential applications of molecular electronics. Ultimately, it is desirable for this technology to operate at around room temperature, and it is therefore important to consider the role of dissipative effects in these conditions. Here, we develop a theory of thermoelectricity which accounts for the vibrational coupling within the framework of the Marcus theory. We demonstrate that the inclusion of lifetime broadening is ne...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1021/acs.jpcc.8b12163

Authors


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Institution:
University of Oxford
Division:
MPLS
Department:
Materials
Oxford college:
Wolfson College
Role:
Author
ORCID:
0000-0003-4104-2664
More by this author
Institution:
University of Oxford
Department:
Materials
Oxford college:
St Anne's College
Role:
Author
ORCID:
0000-0003-0411-2598
More by this author
Role:
Author
ORCID:
0000-0003-1232-9885
Publisher:
American Chemical Society Publisher's website
Journal:
Journal of Physical Chemistry C Journal website
Volume:
123
Issue:
7
Pages:
4103-4108
Publication date:
2019-02-13
Acceptance date:
2019-01-24
DOI:
EISSN:
1932-7455
ISSN:
1932-7447
Source identifiers:
976256
Language:
English
Keywords:
Pubs id:
pubs:976256
UUID:
uuid:f2ce238f-de00-46a7-bb70-e02cb9f199b3
Local pid:
pubs:976256
Deposit date:
2019-02-25

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