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From biomass-derived furans to aromatics with ethanol over zeolite.

Abstract:

We report a novel catalytic conversion of biomass-derived furans and alcohols to aromatics over zeolite catalysts. Aromatics are formed via Diels–Alder cycloaddition with ethylene, which is produced in situ from ethanol dehydration. The use of liquid ethanol instead of gaseous ethylene, as the source of dienophile in this one-pot synthesis, makes the aromatics production much simpler and renewable, circumventing the use of ethylene at high pressure. More importantly, both our experiments and ...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1002/anie.201604108

Authors


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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Inorganic Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Inorganic Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Inorganic Chemistry
Role:
Author
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Engineering and Physical Sciences Research Council More from this funder
China Petroleum and Chemical Corporation More from this funder
Publisher:
Wiley Publisher's website
Journal:
Angewandte Chemie International Edition Journal website
Volume:
55
Issue:
42
Pages:
13061-13066
Publication date:
2016-08-01
Acceptance date:
2016-06-06
DOI:
EISSN:
1521-3773
ISSN:
1433-7851
Pmid:
27490584
Source identifiers:
638484
Language:
English
Keywords:
Pubs id:
pubs:638484
UUID:
uuid:d0f4f17d-5e77-4893-9ea1-a3b4aa708048
Local pid:
pubs:638484
Deposit date:
2017-03-09

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