Journal article
Carrier lifetimes and polaronic mass enhancement in the hybrid halide perovskite CH3NH3PbI3 from multiphonon Fröhlich coupling
- Abstract:
-
We elucidate the nature of the electron-phonon interaction in the archetypal hybrid perovskite CH3NH3PbI3 using ab initio many-body calculations and an exactly solvable model. We demonstrate that electrons and holes near the band edges primarily interact with three distinct groups of longitudinal-optical vibrations, in order of importance: the stretching of the Pb—I bond, the bending of the Pb—I—Pb bonds, and the libration of the organic cations. These pol...
Expand abstract
- Publication status:
- Published
- Peer review status:
- Peer reviewed
Actions
Access Document
- Files:
-
-
(Version of record, pdf, 963.7KB)
-
- Publisher copy:
- 10.1103/physrevlett.121.086402
Why is the content I wish to access not available via ORA?
Bibliographic data (the information relating to research outputs) and full-text items (e.g. articles, theses, reports, etc.) arrive in ORA from several different sources. Unfortunately we are not able to make available the full-text for every research output.
Please contact the ORA team (
) if you have queries regarding unavailable content OR if you are aware of a full-text copy we can make available.
) if you have queries regarding unavailable content OR if you are aware of a full-text copy we can make available.
Content may be unavailable for the following four reasons
-
Version unsuitable
-
We have not obtained a suitable full-text for a given research output. See this page for more information.
-
Recently completed
-
Sometimes content is held in ORA but is unavailable for a fixed period of time to comply with the policies and wishes of rights holders.
-
Permissions
-
All content made available in ORA should comply with relevant rights, such as copyright. See this page for more information.
-
Clearance
-
Some thesis volumes scanned as part of the digitisation scheme funded by Dr Leonard Polonsky are currently unavailable due to sensitive material or uncleared third-party copyright content. We are attempting to contact authors whose theses are affected.
Alternative access to the full-text
You may be able to access the full-text directly from the publisher's website using the 'Publisher Copy' link in the 'Links & Downloads' box from a research output's ORA record page. This method may require an institutional or individual subscription to the journal/resource.
Authors
Funding
Bibliographic Details
- Publisher:
- American Physical Society Publisher's website
- Journal:
- Physical Review Letters Journal website
- Volume:
- 121
- Issue:
- 8
- Article number:
- 086402
- Publication date:
- 2018-08-23
- DOI:
- EISSN:
-
1079-7114
- ISSN:
-
0031-9007
- Pmid:
-
30192620
- Source identifiers:
-
911930
Item Description
- Language:
- English
- Subjects:
- Pubs id:
-
pubs:911930
- UUID:
-
uuid:8e92aeb9-4c8b-414e-92d0-93ce7890ede6
- Local pid:
- pubs:911930
- Deposit date:
- 2019-03-25
Terms of use
- Copyright holder:
- American Physical Society
- Copyright date:
- 2018
- Notes:
- © 2018 American Physical Society
If you are the owner of this record, you can report an update to it here: Report update to this record