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Fungal-derived brevianamide assembly by a stereoselective semipinacolase

Abstract:

Fungal bicyclo[2.2.2]diazaoctane indole alkaloids represent an important family of natural products with a wide spectrum of biological activities. Although biomimetic total syntheses of representative compounds have been reported, the details of their biogenesis, especially the mechanisms for the assembly of diastereomerically distinct and enantiomerically antipodal metabolites, have remained largely uncharacterized. Brevianamide A represents a basic form of the subfamily bearing a dioxopiper...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1038/s41929-020-0454-9

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Publisher:
Nature Research Publisher's website
Journal:
Nature Catalysis Journal website
Volume:
3
Issue:
June 2020
Pages:
497-506
Publication date:
2020-05-18
Acceptance date:
2020-03-16
DOI:
EISSN:
2520-1158
Language:
English
Keywords:
Pubs id:
1107506
Local pid:
pubs:1107506
Deposit date:
2020-07-30

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