Journal article
Visible light photocatalysis of 6π heterocyclization
- Abstract:
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Photo-mediated 6π cyclization is a valuable method for the formation of fused heterocyclic systems. Here we demonstrate that irradiation of cyclic 2-aryloxyketones with blue LED light in the presence of an Ir(III) complex leads to efficient and high yielding arylation across a panoply of substrates by energy transfer. 2-arylthioketones and 2-arylaminoketones also cyclize effectively under these conditions. Quantum calculation demonstrates that the reaction proceeds via conrotatory ring closur...
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- Publication status:
- Published
- Peer review status:
- Peer reviewed
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(Version of record, pdf, 4.2MB)
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- Publisher copy:
- 10.1002/anie.201705333
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Authors
Funding
+ Engineering and Physical Sciences Research Council
More from this funder
Grant:
Medicine(EP/
L015838/1)forstudentships(toN.A.P
Centrefor
DoctoralTraininginSynthesisforBiology
L.V.D
+ Deutsche Forschungsgemeinschaft
More from this funder
Grant:
MU 3987/1-1) for a fellowship (to N.M.
Bibliographic Details
- Publisher:
- Wiley Publisher's website
- Journal:
- Angewandte Chemie Journal website
- Volume:
- 56
- Issue:
- 32
- Pages:
- 9468–9472
- Publication date:
- 2017-07-04
- Acceptance date:
- 2017-06-20
- DOI:
- EISSN:
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1521-3757
- ISSN:
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0044-8249
- Source identifiers:
-
701472
Item Description
- Keywords:
- Pubs id:
-
pubs:701472
- UUID:
-
uuid:2cfee4a2-9d86-4a80-beef-ea01e7085c43
- Local pid:
- pubs:701472
- Deposit date:
- 2017-06-21
Terms of use
- Copyright holder:
- Münster et al
- Copyright date:
- 2017
- Notes:
-
Copyright © 2017 The Authors. Published by Wiley-VCH Verlag GmbH & Co. KGaA.
This is an open access article under the terms of the Creative Commons Attribution License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.
- Licence:
- CC Attribution (CC BY)
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