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Radical pair intersystem crossing: Quantum dynamics or incoherent kinetics?

Abstract:

Magnetic field effects on radical pair reactions arise due to the interplay of coherent electron spin dynamics and spin relaxation effects, a rigorous treatment of which requires the solution of the Liouville-von Neumann equation. However, it is often found that simple incoherent kinetic models of the radical pair singlet-triplet intersystem crossing provide an acceptable description of experimental measurements. In this paper, we outline the theoretical basis for this incoherent kinetic desc...

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Publication status:
Published
Peer review status:
Peer reviewed

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Files:
Publisher copy:
10.1063/1.5095204

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Role:
Author
ORCID:
0000-0003-0625-731X
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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Oxford college:
St Edmund Hall
Role:
Author
ORCID:
0000-0002-7111-0763
Publisher:
AIP Publishing Publisher's website
Journal:
Journal of Chemical Physics Journal website
Volume:
150
Issue:
15
Article number:
151102
Publication date:
2019-04-18
Acceptance date:
2019-04-05
DOI:
EISSN:
1089-7690
ISSN:
0021-9606
Pmid:
31005083
Source identifiers:
995153
Language:
English
Keywords:
Pubs id:
pubs:995153
UUID:
uuid:0378c39e-f3db-4ba3-84ba-d5092bf8cd6e
Local pid:
pubs:995153
Deposit date:
2019-05-27

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