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Facile in situ reductive synthesis of both nitrogen deficient and protonated g-C3N4 nanosheets for the synergistic enhancement of visible-light H2 evolution

Abstract:

A new strategy is reported here to synthesize both nitrogen deficient and protonated graphitic carbon nitride (g-C3N4) nanosheets by the conjoint use of NH4Cl as a dynamic gas template together with hypophosphorous acid (H3PO2) as a doping agent. The NH4Cl treatment allows for the scalable production of protonated g-C3N4 nanosheets. With the corresponding co-addition of H3PO2, nitrogen vacancies, accompanied by both additional protons and interstitially-doped phosphorus, are introduced into t...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1039/c9sc05060d

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Publisher:
Royal Society of Chemistry Publisher's website
Journal:
Chemical Science Journal website
Volume:
11
Issue:
10
Pages:
2716-2728
Publication date:
2020-02-03
Acceptance date:
2020-01-31
DOI:
EISSN:
2041-6539
ISSN:
2041-6520
Language:
English
Keywords:
Pubs id:
1087375
Local pid:
pubs:1087375
Deposit date:
2020-05-11

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